Willard Libby (1908–1980), a professor of chemistry at the University of Chicago, began the research that led him to radiocarbon dating in 1945.
They also sampled artifacts from museums such as a piece of timber from Egyptian pharaoh Senusret III’s funerary boat, an object whose age was known by the record of its owner’s death.
In 1949, Libby and Arnold published their findings in the journal Science, introducing the “Curve of Knowns.” This graph compared the known age of artifacts with the estimated age as determined by the radiocarbon dating method.
Finally, Libby had a method to put his concept into practice. The circular arrangement of Geiger counters (center) detected radiation in samples while the thick metal shields on all sides were designed to reduce background radiation.
The concept of radiocarbon dating relied on the ready assumption that once an organism died, it would be cut off from the carbon cycle, thus creating a time-capsule with a steadily diminishing carbon-14 count.
Libby and graduate student Ernest Anderson (1920–2013) calculated the mixing of carbon across these different reservoirs, particularly in the oceans, which constitute the largest reservoir.